Through the Azure portal I can disconnect my VNet integration, see below. I need to do this in a Powershell script, using the Az module. Is this possible?

Just use the command below, it works fine on my side.
Remove-AzResource -ResourceGroupName "<resource-group-name>" -ResourceType "Microsoft.Web/sites/config" -ResourceName "<webapp-name>/virtualNetwork" -Force
Or
Remove-AzResource -ResourceId "/subscriptions/<subscription-id>/resourceGroups/<resource-group-name>/providers/Microsoft.Web/sites/<webapp-name>/config/virtualNetwork" -Force
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